Visible-infrared two-dimensional Fourier-transform spectroscopy

Nadia Belabas (1) , Manuel Joffre (1)

1 LOB - Laboratoire d'optique et biosciences

We report on a new class of optical multidimensional Fourier-transform spectroscopy associated with a visible excitation-infrared emission configuration, in which the emitted field results from second-order optical nonlinearities. This configuration is demonstrated on a phase-matched sample of known nonlinear response by coherent measurement of the mid-infrared field emitted after a femtosecond visible double-pulse excitation. (C) 2002 Optical Society of America.

Domaines: Optique [physics.optics]

Nadia Belabas, Manuel Joffre. Visible-infrared two-dimensional Fourier-transform spectroscopy. Optics Letters, 2002, 27 (22), pp.2043. ⟨10.1364/OL.27.002043⟩. ⟨hal-00837024⟩