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Nonlinear optical activity in chiral molecules: Surface second harmonic generation and nonlinear circular dichroism
Abstract : Nonlinear optical activity in chiral molecules is investigated. We first examine the importance of the nonlocality of the light-matter interaction in optical activity and extend this concept to second-order (surface second harmonic generation) and third-order (nonlinear circular dichroism) nonlinear optical phenomena. Microscopic models are also discussed. Various phenomena derived from these considerations are demonstrated experimentally with specially-synthesized chiral molecules. Cop. 2002 Académie des sciences/Éditions scientifiques et médicales Elsevier SAS.
https://hal-polytechnique.archives-ouvertes.fr/hal-00836937
Contributor : Denis Roura <>
Submitted on : Tuesday, June 25, 2013 - 9:16:43 PM
Last modification on : Friday, June 18, 2021 - 3:58:03 PM
Contributor : Denis Roura <>
Submitted on : Tuesday, June 25, 2013 - 9:16:43 PM
Last modification on : Friday, June 18, 2021 - 3:58:03 PM