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Visible-infrared two-dimensional Fourier-transform spectroscopy

Abstract : We report on a new class of optical multidimensional Fourier-transform spectroscopy associated with a visible excitation-infrared emission configuration, in which the emitted field results from second-order optical nonlinearities. This configuration is demonstrated on a phase-matched sample of known nonlinear response by coherent measurement of the mid-infrared field emitted after a femtosecond visible double-pulse excitation. (C) 2002 Optical Society of America.
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Nadia Belabas, Manuel Joffre. Visible-infrared two-dimensional Fourier-transform spectroscopy. Optics Letters, Optical Society of America - OSA Publishing, 2002, 27 (22), pp.2043. ⟨10.1364/OL.27.002043⟩. ⟨hal-00837024⟩



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